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Review of results of theoretical approaches to phonon engineering of thermodynamic properties for different quantum structures

Pregled rezultata teorijskih pristupa fononskom inženjeringu termodinamičkih osobina različitih kvantnih struktura

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2015
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Jaćimovski, Stevo
Šetrajčić, Jovan P.
Article (Published version)
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Abstract
Application of nano-structures requires a knowledge of their fundamental physical (mechanical, electro-magnetic, optical, etc.) characteristics. Thermodynamic properties associated with phonon displacements through the nanosamples are particularly interesting. Independent of the type of lattices, the thermodynamics of their subsystems (electrons, excitons, spin waves, etc.) is determined when the subsystem is in thermodynamic equilibrium with phonons. Phonons are collective mechanical oscillations of molecules or atoms and represent the most important system of excitations. Besides, the acoustical characteristics as well as conductive and superconductive properties etc. could not be realistically explained without phonons. In this paper we will try to observe the difference between the characteristics of different nano-crystalline structures: ultrathin films, composite films, i.e. superlattices, nanorods and quantum dots, we were interested in whether the quantum size effects (quantum ...confinement), quantum (de)coherence and influence of boundary conditions, strengthen or weaken in nanosamples. Finally, this paper describes how the dimensional confinement of phonons in nanostructures leads to modifications in the electronic, optical, acoustic, superconducting and thermodynamic properties of quantum. Thermal properties of nanostructures have recently attracted a lot of attention. The influence of size effects on thermal conductivity is becoming extremely important for device design and reliability. On the basis of the calculated dispersion law and distribution of phonon states in nanoscopic crystals, free energy and entropy will be calculated. Internal energy as well as heat capacitance will also be analyzed.

Primena naostruktura zhteva poznavanje njihovih osnovnih fizičkih (mehaničkih, elektromagnetnih, optičkih, itd.) karakteristika. Termodinamičke osobine su povezane sa ponašanjem fononskog podsistema koji uvek postoji. Fononi su kolektivne mehaničke oscilacije molekula ili atoma kristalne rešetke i predstavljaju najvažniji sistem ekscitacija u ovim strukturama.Nezavisno od tipa kristalne rešetke termodinamika njenih podsistema (elektrona, eksitona, spinskih talasa itd.) je određena kada je odgovarajući podsistem u termodinamičkoj ravnoteži sa fononima. Uloga fonona u nanostrukturama je značajnija nego u tzv. balk strukturama, posebno što je u nanostrukturama (filmovi, superrešetke, žice, tačke) kretanje fonona ograničeno u nekoliko dimenzija. Zbog ograničenosti dimenzija kod nanostruktura se javljaju novi efekti kao što je dimenziono kvantovanje, konfiniranje fonona itd. Uticaj graničnih uslova na zakon disperzije fonona dovodi do promene karakteristika termodinamičkih i transportnih os...obina. Dakle, menjanjem graničnih uslova se može uticati na toplotne i transportne osobine ovih struktura, što se danas popularno naziva fononski inženjering. U radu su analizirani i upoređivani toplotni kapaciteti i koficijenti toplotne provodnosti (kao merljive veličine) za razne strukture, kako na niskim tako i na visokim temperaturama, kao i posledice na njihovu praktičnu primenu.

Keywords:
phonons / Green's function / ultrathin films / superlattices / quantum wires-nanorods / quantum dots / energy spectra / thermodynamic behavior / specific heat / thermal conductivity
Source:
Nauka, bezbednost, policija, 2015, 20, 3, 67-82
Publisher:
  • Kriminalističko- policijska akademija, Beograd
Funding / projects:
  • Design and modeling of specific features of nanostructured samples (RS-171039)
  • Inovation of Forensic Methods and their Application (RS-34019)

DOI: 10.5937/NBP1503067J

ISSN: 0354-8872

[ Google Scholar ]
URI
http://jakov.kpu.edu.rs/handle/123456789/625
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  • Radovi istraživača / Researchers' publications
Institution/Community
Jakov
TY  - JOUR
AU  - Jaćimovski, Stevo
AU  - Šetrajčić, Jovan P.
PY  - 2015
UR  - http://jakov.kpu.edu.rs/handle/123456789/625
AB  - Application of nano-structures requires a knowledge of their fundamental physical (mechanical, electro-magnetic, optical, etc.) characteristics. Thermodynamic properties associated with phonon displacements through the nanosamples are particularly interesting. Independent of the type of lattices, the thermodynamics of their subsystems (electrons, excitons, spin waves, etc.) is determined when the subsystem is in thermodynamic equilibrium with phonons. Phonons are collective mechanical oscillations of molecules or atoms and represent the most important system of excitations. Besides, the acoustical characteristics as well as conductive and superconductive properties etc. could not be realistically explained without phonons. In this paper we will try to observe the difference between the characteristics of different nano-crystalline structures: ultrathin films, composite films, i.e. superlattices, nanorods and quantum dots, we were interested in whether the quantum size effects (quantum confinement), quantum (de)coherence and influence of boundary conditions, strengthen or weaken in nanosamples. Finally, this paper describes how the dimensional confinement of phonons in nanostructures leads to modifications in the electronic, optical, acoustic, superconducting and thermodynamic properties of quantum. Thermal properties of nanostructures have recently attracted a lot of attention. The influence of size effects on thermal conductivity is becoming extremely important for device design and reliability. On the basis of the calculated dispersion law and distribution of phonon states in nanoscopic crystals, free energy and entropy will be calculated. Internal energy as well as heat capacitance will also be analyzed.
AB  - Primena naostruktura zhteva poznavanje njihovih osnovnih fizičkih (mehaničkih, elektromagnetnih, optičkih, itd.) karakteristika. Termodinamičke osobine su povezane sa ponašanjem fononskog podsistema koji uvek postoji. Fononi su kolektivne mehaničke oscilacije molekula ili atoma kristalne rešetke i predstavljaju najvažniji sistem ekscitacija u ovim strukturama.Nezavisno od tipa kristalne rešetke termodinamika njenih podsistema (elektrona, eksitona, spinskih talasa itd.) je određena kada je odgovarajući podsistem u termodinamičkoj ravnoteži sa fononima. Uloga fonona u nanostrukturama je značajnija nego u tzv. balk strukturama, posebno što je u nanostrukturama (filmovi, superrešetke, žice, tačke) kretanje fonona ograničeno u nekoliko dimenzija. Zbog ograničenosti dimenzija kod nanostruktura se javljaju novi efekti kao što je dimenziono kvantovanje, konfiniranje fonona itd. Uticaj graničnih uslova na zakon disperzije fonona dovodi do promene karakteristika termodinamičkih i transportnih osobina. Dakle, menjanjem graničnih uslova se može uticati na toplotne i transportne osobine ovih struktura, što se danas popularno naziva fononski inženjering. U radu su analizirani i upoređivani toplotni kapaciteti i koficijenti toplotne provodnosti (kao merljive veličine) za razne strukture, kako na niskim tako i na visokim temperaturama, kao i posledice na njihovu praktičnu primenu.
PB  - Kriminalističko- policijska akademija, Beograd
T2  - Nauka, bezbednost, policija
T1  - Review of results of theoretical approaches to phonon engineering of thermodynamic properties for different quantum structures
T1  - Pregled rezultata teorijskih pristupa fononskom inženjeringu termodinamičkih osobina različitih kvantnih struktura
VL  - 20
IS  - 3
SP  - 67
EP  - 82
DO  - 10.5937/NBP1503067J
UR  - conv_168
ER  - 
@article{
author = "Jaćimovski, Stevo and Šetrajčić, Jovan P.",
year = "2015",
abstract = "Application of nano-structures requires a knowledge of their fundamental physical (mechanical, electro-magnetic, optical, etc.) characteristics. Thermodynamic properties associated with phonon displacements through the nanosamples are particularly interesting. Independent of the type of lattices, the thermodynamics of their subsystems (electrons, excitons, spin waves, etc.) is determined when the subsystem is in thermodynamic equilibrium with phonons. Phonons are collective mechanical oscillations of molecules or atoms and represent the most important system of excitations. Besides, the acoustical characteristics as well as conductive and superconductive properties etc. could not be realistically explained without phonons. In this paper we will try to observe the difference between the characteristics of different nano-crystalline structures: ultrathin films, composite films, i.e. superlattices, nanorods and quantum dots, we were interested in whether the quantum size effects (quantum confinement), quantum (de)coherence and influence of boundary conditions, strengthen or weaken in nanosamples. Finally, this paper describes how the dimensional confinement of phonons in nanostructures leads to modifications in the electronic, optical, acoustic, superconducting and thermodynamic properties of quantum. Thermal properties of nanostructures have recently attracted a lot of attention. The influence of size effects on thermal conductivity is becoming extremely important for device design and reliability. On the basis of the calculated dispersion law and distribution of phonon states in nanoscopic crystals, free energy and entropy will be calculated. Internal energy as well as heat capacitance will also be analyzed., Primena naostruktura zhteva poznavanje njihovih osnovnih fizičkih (mehaničkih, elektromagnetnih, optičkih, itd.) karakteristika. Termodinamičke osobine su povezane sa ponašanjem fononskog podsistema koji uvek postoji. Fononi su kolektivne mehaničke oscilacije molekula ili atoma kristalne rešetke i predstavljaju najvažniji sistem ekscitacija u ovim strukturama.Nezavisno od tipa kristalne rešetke termodinamika njenih podsistema (elektrona, eksitona, spinskih talasa itd.) je određena kada je odgovarajući podsistem u termodinamičkoj ravnoteži sa fononima. Uloga fonona u nanostrukturama je značajnija nego u tzv. balk strukturama, posebno što je u nanostrukturama (filmovi, superrešetke, žice, tačke) kretanje fonona ograničeno u nekoliko dimenzija. Zbog ograničenosti dimenzija kod nanostruktura se javljaju novi efekti kao što je dimenziono kvantovanje, konfiniranje fonona itd. Uticaj graničnih uslova na zakon disperzije fonona dovodi do promene karakteristika termodinamičkih i transportnih osobina. Dakle, menjanjem graničnih uslova se može uticati na toplotne i transportne osobine ovih struktura, što se danas popularno naziva fononski inženjering. U radu su analizirani i upoređivani toplotni kapaciteti i koficijenti toplotne provodnosti (kao merljive veličine) za razne strukture, kako na niskim tako i na visokim temperaturama, kao i posledice na njihovu praktičnu primenu.",
publisher = "Kriminalističko- policijska akademija, Beograd",
journal = "Nauka, bezbednost, policija",
title = "Review of results of theoretical approaches to phonon engineering of thermodynamic properties for different quantum structures, Pregled rezultata teorijskih pristupa fononskom inženjeringu termodinamičkih osobina različitih kvantnih struktura",
volume = "20",
number = "3",
pages = "67-82",
doi = "10.5937/NBP1503067J",
url = "conv_168"
}
Jaćimovski, S.,& Šetrajčić, J. P.. (2015). Review of results of theoretical approaches to phonon engineering of thermodynamic properties for different quantum structures. in Nauka, bezbednost, policija
Kriminalističko- policijska akademija, Beograd., 20(3), 67-82.
https://doi.org/10.5937/NBP1503067J
conv_168
Jaćimovski S, Šetrajčić JP. Review of results of theoretical approaches to phonon engineering of thermodynamic properties for different quantum structures. in Nauka, bezbednost, policija. 2015;20(3):67-82.
doi:10.5937/NBP1503067J
conv_168 .
Jaćimovski, Stevo, Šetrajčić, Jovan P., "Review of results of theoretical approaches to phonon engineering of thermodynamic properties for different quantum structures" in Nauka, bezbednost, policija, 20, no. 3 (2015):67-82,
https://doi.org/10.5937/NBP1503067J .,
conv_168 .

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